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Theoretical and Empirical Studies on the Catalytic Partial Oxidation of Methane Promoted by FeY and Fe(piperazine)Y Complexes (Y = Y-zeolite)
1Universidade Estadual de Maringá, email@example.com
2Universidade Estadual de Maringá, firstname.lastname@example.org
3Universidade Federal do Rio de Janeiro, email@example.com
4Universidade Estadual de Maringá, firstname.lastname@example.org
5Universidade Tiradentes, email@example.com
6Universidade Estadual do Norte Fluminense, firstname.lastname@example.org
7Universidade Estadual de Maringá, email@example.com
Citation Information: International Journal of Chemical Reactor Engineering. Volume 9, Issue 1, Pages –, ISSN (Online) 1542-6580, DOI: 10.2202/1542-6580.2381, November 2011
- Published Online:
In this study, we synthesized and characterized zeolite-encapsulated Fe(III) complexes containing piperazine-derived ligands. The catalytic activity of these complexes was tested in the partial oxidation of methane to methanol using O2 as a low-pressure oxidant. Values for methane conversion of up to 1.2% with methanol selectivity of up to 6.7% were obtained. The experimental data were compared with thermodynamic simulation results for the reaction that takes place as a basic principle, the minimization of Gibbs free energy.