Jump to ContentJump to Main Navigation
Show Summary Details
More options …

Open Chemistry

formerly Central European Journal of Chemistry

1 Issue per year


IMPACT FACTOR 2016 (Open Chemistry): 1.027
IMPACT FACTOR 2016 (Central European Journal of Chemistry): 1.460

CiteScore 2016: 0.61

SCImago Journal Rank (SJR) 2016: 0.288
Source Normalized Impact per Paper (SNIP) 2016: 0.735

Open Access
Online
ISSN
2391-5420
See all formats and pricing
More options …
Volume 11, Issue 11

Issues

Chemical modification and characterization of poly(ethylene terephthalate) surfaces for collagen immobilization

Mioara Drobota / Zdenka Persin
  • Laboratory for Characterization and Processing of Polymers, Faculty of Mechanical Engineering, Institute for Engineering Materials and Design, University of Maribor, SI-2000, Maribor, Slovenia
  • Centre of Excellence for Polymer Materials and Technologies, SI-1000, Ljubljana, Slovenia
  • Email
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Lidija Zemljic
  • Laboratory for Characterization and Processing of Polymers, Faculty of Mechanical Engineering, Institute for Engineering Materials and Design, University of Maribor, SI-2000, Maribor, Slovenia
  • Email
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Tamiselvan Mohan
  • Laboratory for Characterization and Processing of Polymers, Faculty of Mechanical Engineering, Institute for Engineering Materials and Design, University of Maribor, SI-2000, Maribor, Slovenia
  • Email
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Karin Stana-Kleinschek
  • Laboratory for Characterization and Processing of Polymers, Faculty of Mechanical Engineering, Institute for Engineering Materials and Design, University of Maribor, SI-2000, Maribor, Slovenia
  • Centre of Excellence for Polymer Materials and Technologies, SI-1000, Ljubljana, Slovenia
  • Email
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Ales Doliska
  • Laboratory for Characterization and Processing of Polymers, Faculty of Mechanical Engineering, Institute for Engineering Materials and Design, University of Maribor, SI-2000, Maribor, Slovenia
  • Centre of Excellence for Polymer Materials and Technologies, SI-1000, Ljubljana, Slovenia
  • Email
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Matej Bracic
  • Laboratory for Characterization and Processing of Polymers, Faculty of Mechanical Engineering, Institute for Engineering Materials and Design, University of Maribor, SI-2000, Maribor, Slovenia
  • Email
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Volker Ribitsch / Valeria Harabagiu / Sergiu Coseri
Published Online: 2013-08-25 | DOI: https://doi.org/10.2478/s11532-013-0319-z

Abstract

The functionalization of poly(ethylene terephthalate) (PET) surface films by reactions with multifunctional amines such as triethylenetetramine (TETA), and tetraethylenepentamine (TEPA) was investigated. For the functionalization of PET films surface we used a new way of treatment, a “sandwich model”. Physical-chemical properties of functionalized PET films were analysed. Qualitative and quantitative determination of the introduced amine groups were examined by means of Fourier Transform Infrared Attenuated Total Reflexion (FTIR — ATR), X-ray photoelectron spectroscopy (XPS), and potentiometric titration. Gained wetting properties were determined by using contact angle measurements and thoroughly analysed by acid-base approach. In addition, surface topography was investigated by atomic force microscopy (AFM). The amount of the introduced amino groups after TETA incorporation has been found to be two times higher as compared to TEPA. Wetting properties were significantly improved after aminolysis. Surface free energy was higher for PET — TETA treated film than that observed for PET — TEPA treated which is in accordance with titration results. The collagen immobilization onto PET treated films was evidenced by using AFM and subsequently by using XPS.

Keywords: PET; Aminolysis; Wettability; AFM; Collagen immobilization

  • [1] R.J. Good, In: R.J. Good, R.R. Stromberg (Eds.), Surface and Colloid Science (Plenum Press, New York, 1979) CrossrefGoogle Scholar

  • [2] J. Mayingi, G. Hélary, F. Noirclere, B. Bacroix, V. Migonney, ITBM-RBM. 29, 1 (2008) Google Scholar

  • [3] K.S. Iyer, I. Luzinov, Macromolecules 37, 9538 (2004) http://dx.doi.org/10.1021/ma0493168CrossrefGoogle Scholar

  • [4] S. Coseri, G. Nistor, L. Fras, S. Strnad, V. Harabagiu, B.C. Simionescu, Biomacromolecules 10, 2294 (2009) http://dx.doi.org/10.1021/bm9004854CrossrefGoogle Scholar

  • [5] G. Biliuta, L. Fras, S. Strnad, V. Harabagiu, S. Coseri, J. Polym. Sci, Part A: Polym. Chem. 48, 4790 (2010) http://dx.doi.org/10.1002/pola.24270CrossrefGoogle Scholar

  • [6] M. Geoghegan, G. Krausch, Prog. Polym. Sci. 28, 261 (2003) http://dx.doi.org/10.1016/S0079-6700(02)00080-1CrossrefGoogle Scholar

  • [7] M.H. Kunita, E.M. Girotto, E.C. Muniz, A.F. Rubira, Braz. J. Chem. Eng. 23, 267 (2006) http://dx.doi.org/10.1590/S0104-66322006000200015CrossrefGoogle Scholar

  • [8] C. Zhang, N. Luo, D.E. Hirt, Langmuir 22, 6851 (2006) http://dx.doi.org/10.1021/la0532712CrossrefGoogle Scholar

  • [9] N. Luo, J.B. Hutchison, K.S. Anseth, C.N. Bowman, Macromolecules 35, 2487 (2002) http://dx.doi.org/10.1021/ma011487eCrossrefGoogle Scholar

  • [10] B.P. Harris, A.T. Metters, Macromolecules 39, 2764 (2006) http://dx.doi.org/10.1021/ma0512051CrossrefGoogle Scholar

  • [11] P. Yang, X. Zhang, J.Y. Xie, J.C. Chen, W.T. Yang, Biomacromolecules 7, 2770 (2006) http://dx.doi.org/10.1021/bm0605356CrossrefGoogle Scholar

  • [12] Y. Liu, H.J. Lu, W. Zhong, P.Y. Song, J.L. Kong, P.Y. Yang, H.H. Girault, B.H. Liu, Anal. Chem. 78, 801 (2006) http://dx.doi.org/10.1021/ac051463wCrossrefGoogle Scholar

  • [13] J. Fu, J. Ji, D. Fan, J. Shen, J Biomed. Mater. Res. A. 79, 665 (2006) CrossrefGoogle Scholar

  • [14] J. Fu, J. Ji, W. Yuan, J. Shen, Biomaterials 26, 6684 (2005) http://dx.doi.org/10.1016/j.biomaterials.2005.04.034CrossrefGoogle Scholar

  • [15] X.S. Jiang, C.H. Chai, Y. Zhang, R. Zhuo, H.Q. Mao, K.W. Leong, Biomaterials 27, 2723 (2006) http://dx.doi.org/10.1016/j.biomaterials.2005.12.001CrossrefGoogle Scholar

  • [16] T. Brueckner, A. Eberl, S. Heumann, M. Rabe, G.M. Guebitz, J Polym Sci, Part A: Polym. Chem. 46, 6435 (2008) http://dx.doi.org/10.1002/pola.22952CrossrefGoogle Scholar

  • [17] W. Zhang, X. Yi, X. Sun, Y. Zhang, Chem. Technol. Biotechnol. 83, 904 (2008) http://dx.doi.org/10.1002/jctb.1890CrossrefGoogle Scholar

  • [18] X. Li, J. Ji, M. Pu, X. Wang, J. Shen, J. Mater. Sci. Mater. Med. 19, 291 (2008) http://dx.doi.org/10.1007/s10856-006-0110-1CrossrefGoogle Scholar

  • [19] E. Rusu, M. Drobota, V. Barboiu, J. Optoelectron Adv. Mater. 10, 377 (2008) Google Scholar

  • [20] Q. Feng, C. Chai, X.S. Jiang, K.W. Leong, H.Q. Mao, J Biomed. Mater. Res. A. 78, 781 (2006) CrossrefGoogle Scholar

  • [21] Y. Zhang, C. Chai, X.S. Jiang, S.H. Teoh, K.W. Leog, Mater. Sci. Eng. 27, 213 (2007) http://dx.doi.org/10.1016/j.msec.2006.03.013CrossrefGoogle Scholar

  • [22] T. Ohe, Y. Yoshimura, I. Abe, M. Ikeda, Y. Shibutani, Textile Res. J. 77, 131 (2007) http://dx.doi.org/10.1177/0040517507076325CrossrefGoogle Scholar

  • [23] L. Bech, T. Meylheuc, B. Lepoittevin, P. Roger, J Polym Sci, Part A: Polym. Chem. 45, 2172 (2007) http://dx.doi.org/10.1002/pola.21983CrossrefGoogle Scholar

  • [24] V.T. Bhat, N.R. James, A. Jayakrishnan, Polym. Int. 57, 124 (2008) http://dx.doi.org/10.1002/pi.2332CrossrefGoogle Scholar

  • [25] E.Y. Kim, J.S. Kong, S.K. An, H.D. Kim, J. Adhes. Sci. Technol. 14, 1119 (2000) http://dx.doi.org/10.1163/156856100743121CrossrefGoogle Scholar

  • [26] S.L. Favaro, A.F. Rubira, E.C. Muniz, E. Radovanovic, Polym. Degrad. Stab. 92, 1219 (2007) http://dx.doi.org/10.1016/j.polymdegradstab.2007.04.005CrossrefGoogle Scholar

  • [27] M.H. Zohdy, Radiat. Phys. Chem. 73, 101 (2005) http://dx.doi.org/10.1016/j.radphyschem.2004.07.002CrossrefGoogle Scholar

  • [28] K.S. Chen, Y.A. Ku, H.R. Lin. Hong-Ru Lin, T.R. Yan, D.C. Sheu, T.M. Chen, J. Appl. Polym. Sci. 100, 803 (2006) http://dx.doi.org/10.1002/app.23111CrossrefGoogle Scholar

  • [29] J.P. Chen, Y.P. Chiang, J. Membr. Sci. 270, 212 (2006) http://dx.doi.org/10.1016/j.memsci.2005.11.015CrossrefGoogle Scholar

  • [30] P.S. Curti, M.R. Moura, W. Veiga, E. Radovanovic., A.F. Rubira, E.C. Muniz, Appl. Surf. Sci. 245, 223 (2005) http://dx.doi.org/10.1016/j.apsusc.2004.10.019CrossrefGoogle Scholar

  • [31] M. Ciobanu, A. Siove, V. Gueguen, L.J. Gamble, D.G. Castner, V. Migonney, Biomacromolecules 7, 755 (2006) http://dx.doi.org/10.1021/bm050694+CrossrefGoogle Scholar

  • [32] Y. Liu, G. Wu, L. Gu, AATCC. Rev. 8, 44 (2008) Google Scholar

  • [33] G. Pavon-Djavid, L.J. Gamble, M. Ciobanu, V. Gueguen, D.G. Castner, V. Migonney, Biomacromolecules 8, 3317 (2007) http://dx.doi.org/10.1021/bm070344iCrossrefGoogle Scholar

  • [34] N. Singh, A.W. Bridges, A.J. Garcia, L.A. Lyon, Biomacromolecules 8, 3271 (2007) http://dx.doi.org/10.1021/bm700516vCrossrefGoogle Scholar

  • [35] C.H. Jou, S.M. Lin, L. Yun, M.C. Hwang, D.G. Yu3, W.L. Chou, J.S. Lee, M.C. Yang, Polym. Adv. Technol. 18, 235 (2007) http://dx.doi.org/10.1002/pat.866Google Scholar

  • [36] C.H. Jou, L. Yuan, S.M. Lin, M.C. Hwang, W.L. Chou, D.G. Yu, M.C. Yang, J. Appl. Polym. Sci. 104, 220 (2007) http://dx.doi.org/10.1002/app.25549CrossrefGoogle Scholar

  • [37] H.G. Hicke, M. Becker, B.R. Paulke, M. Ulbricht, J. Membr. Sci. 282, 413 (2006) http://dx.doi.org/10.1016/j.memsci.2006.05.051CrossrefGoogle Scholar

  • [38] A.P. Zhu, F. Zhao, N. Fang, J. Biomed. Mater. Res. A. 86, 467 (2008) CrossrefGoogle Scholar

  • [39] A. Laskarakis, S. Logothetidis, S. Kassavetis, E. Papaioannou, Thin Solid Films 516, 1443 (2008) http://dx.doi.org/10.1016/j.tsf.2007.03.170CrossrefGoogle Scholar

  • [40] I. Topala, N. Dumitrascu, V. Pohoata, Plasma Chem. Plasma Process 27, 95 (2007) http://dx.doi.org/10.1007/s11090-006-9046-yCrossrefGoogle Scholar

  • [41] I. Topala, N. Dumitrascu, V. Pohoata, Plasma Chem. Plasma Process. 28, 535 (2008) http://dx.doi.org/10.1007/s11090-008-9136-0CrossrefGoogle Scholar

  • [42] R. Morent, N.D. Deyter, C. Leys, L. Gengembre, E. Payen, Text Res. J. 77, 471 (2007) http://dx.doi.org/10.1177/0040517507080616CrossrefGoogle Scholar

  • [43] P. Esena, S. Zanini, C. Riccardi, Vacuum 82, 232 (2008) http://dx.doi.org/10.1016/j.vacuum.2007.07.054CrossrefGoogle Scholar

  • [44] S. Zanini, P. Massini, M. Mietta, E. Grimoldi, C. Riccardi, J. Colloid Interface Sci. 322, 566 (2008) http://dx.doi.org/10.1016/j.jcis.2008.04.012CrossrefGoogle Scholar

  • [45] Y. Kurihara, H. Ohata, M. Kawaguchi, S. Yamazaki, K. Kimura, J. Appl. Polym. Sci. 108, 85 (2008) http://dx.doi.org/10.1002/app.27537CrossrefGoogle Scholar

  • [46] G. Farrow, D.A.S. Ravens, I.M. Ward., Polymer 3, 17 (1962) http://dx.doi.org/10.1016/0032-3861(62)90062-9CrossrefGoogle Scholar

  • [47] G.E. Sweet, J.P. Bell, J. Polym. Sci. Part B: Polym Phys 16, 1935 (1978) http://dx.doi.org/10.1002/pol.1978.180161104CrossrefGoogle Scholar

  • [48] G.C. Adams, Polym. Eng. Sci. 16, 222 (1976) http://dx.doi.org/10.1002/pen.760160317CrossrefGoogle Scholar

  • [49] S.A. Holmes, J. Appl. Polym. Sci. 61, 255 (1996) http://dx.doi.org/10.1002/(SICI)1097-4628(19960711)61:2<255::AID-APP7>3.0.CO;2-OCrossrefGoogle Scholar

  • [50] M.H. Kish, S. Borhani, J. Appl. Polym. Sci. 78, 1923 (2000) http://dx.doi.org/10.1002/1097-4628(20001209)78:11<1923::AID-APP110>3.0.CO;2-UCrossrefGoogle Scholar

  • [51] L. Bech, T. Meylheuc, B. Lepoittevin, P. Roger, J Polym Sci, Part A: Polym Chem 45, 2172 (2007) http://dx.doi.org/10.1002/pola.21983CrossrefGoogle Scholar

  • [52] K.E. Nissen, B.H. Stuart, M.G. Stevens, A.T. Baker, J. Polym Sci, Part B: Polym. Phys. 39, 623 (2001) http://dx.doi.org/10.1002/1099-0488(20010315)39:6<623::AID-POLB1036>3.0.CO;2-7CrossrefGoogle Scholar

  • [53] C.D. Volpe, D. Maniglio, M. Brugnara, S. Siboni, M. Morra, J. Colloid Interface Sci. 271, 434 (2004) http://dx.doi.org/10.1016/j.jcis.2003.09.049CrossrefGoogle Scholar

  • [54] C.D. Volpe, S. Siboni, J. Colloid Interface Sci. 195, 121 (1997) http://dx.doi.org/10.1006/jcis.1997.5124CrossrefGoogle Scholar

  • [55] C.J. van Oss, Interfacial Forces in Aqueous Media (Dekker, New York, 1994) Google Scholar

  • [56] K. Herzog, R.J. Müller, W.D. Decker, Polym. Degrad. Stab. 91, 2486 (2006) http://dx.doi.org/10.1016/j.polymdegradstab.2006.03.005CrossrefGoogle Scholar

  • [57] K.C. Cole, J. Guevremont, A. Ajji, M.M. Dumoulin, Appl. Spectrosc. 48, 1513 (1994) http://dx.doi.org/10.1366/0003702944027877CrossrefGoogle Scholar

  • [58] S.K. Bahl, D.D. Cornell, F.J. Boerio, J. Polym. Sci. Polym. Lett. 12, 13 (1974) http://dx.doi.org/10.1002/pol.1974.130120103CrossrefGoogle Scholar

  • [59] R.A. Antonino, S. Elena, B. Ruggero, R. Claudia, F. Orsinic, G. Polettic, L. Medad, M.R. Massafrae, B. Marcandalli, Appl Surf Sci 252, 2265 (2006) http://dx.doi.org/10.1016/j.apsusc.2005.04.013CrossrefGoogle Scholar

  • [60] D.R. Eyre, M.A. Paz, P.M. Gallop, Annu Rev. Biochem. 53, 717 (1984) http://dx.doi.org/10.1146/annurev.bi.53.070184.003441CrossrefGoogle Scholar

  • [61] K. Sokolov, J. Galvan, A. Myakov, A. Lacy, R. Lotan, R. Richards-Kortum, J. Biomed Optic 7, 148 (2002) http://dx.doi.org/10.1117/1.1427052CrossrefGoogle Scholar

  • [62] N. Qureshi, E.V. Stepanov, D. Schiraldi, A. Hiltner. E. Baer, J Polym Sci, Part B: Polym Phys 38, 1679 (2000) http://dx.doi.org/10.1002/1099-0488(20000701)38:13<1679::AID-POLB10>3.0.CO;2-PCrossrefGoogle Scholar

  • [63] M. Dobromir, G. Biliuta, D. Luca, M. Aflori, V. Harabagiu, S. Coseri, Colloids Surf., A 381, 106 (2011) http://dx.doi.org/10.1016/j.colsurfa.2011.03.030CrossrefGoogle Scholar

  • [64] R.A.N. Perile, F.K. Andrade, C. Alves Jr., M. Gama, Carbohydr. Polym. 82, 692 (2010) http://dx.doi.org/10.1016/j.carbpol.2010.05.037CrossrefGoogle Scholar

About the article

Published Online: 2013-08-25

Published in Print: 2013-11-01


Citation Information: Open Chemistry, Volume 11, Issue 11, Pages 1786–1798, ISSN (Online) 2391-5420, DOI: https://doi.org/10.2478/s11532-013-0319-z.

Export Citation

© 2013 Versita Warsaw. This work is licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 3.0 License. BY-NC-ND 3.0

Comments (0)

Please log in or register to comment.
Log in