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Pure and Applied Chemistry

The Scientific Journal of IUPAC

Ed. by Burrows, Hugh / Weir, Ron / Stohner, Jürgen

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Volume 72, Issue 7 (Jan 2000)

Issues

Atom efficiency and catalysis in organic synthesis

Roger A. Sheldon
  • Corresponding author
  • Delft University of Technology, Organic Chemistry and Catalysis, Julianalaan 136, 2628 BL Delft, The Netherlands
  • Other articles by this author:
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Published Online: 2009-01-01 | DOI: https://doi.org/10.1351/pac200072071233

The key to waste minimization in fine chemicals manufacture is the widespread substitution of classical organic syntheses employing stoichiometric amounts of inorganic reagents with cleaner, catalytic alternatives. The E factors (by waste per kg product) of chemical processes increase dramatically on going downstream from bulk to fine chemicals and pharmaceuticals, mainly owing to the use of "stoichiometric" methods. The concept of atom efficiency is a useful tool for rapid evaluation of the amount of waste generated by alternative processes. The general theme of atom-efficient, catalytic processes is illustrated with industrially relevant examples. These include catalysis by solid acids and bases, catalytic reductions and oxidations, catalytic C_C bond formation, asymmetric catalysis, biocatalysis, and catalysis in novel media (aqueous and fluorous biphasic systems, supercritical fluids, and ionic liquids).

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Published Online: 2009-01-01

Published in Print: 2000-01-01


Citation Information: Pure and Applied Chemistry, ISSN (Online) 1365-3075, ISSN (Print) 0033-4545, DOI: https://doi.org/10.1351/pac200072071233.

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Green Chemistry, 2005, Volume 7, Number 3, Page 121
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Advanced Synthesis & Catalysis, 2004, Volume 346, Number 12, Page 1429
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Green Chemistry, 2007, Volume 9, Number 10, Page 1126
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Angewandte Chemie International Edition, 2007, Volume 46, Number 45, Page 8593
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Angewandte Chemie International Edition, 2007, Volume 46, Number 29, Page 5583
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Angewandte Chemie, 2007, Volume 119, Number 29, Page 5679
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Advanced Synthesis & Catalysis, 2007, Volume 349, Number 8-9, Page 1289
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Applied Microbiology and Biotechnology, 2006, Volume 73, Number 5, Page 1087

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