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In This Section
Volume 72, Issue 7 (Jan 2000)

Issues

Atom efficiency and catalysis in organic synthesis

Roger A. Sheldon
  • Corresponding author
  • Delft University of Technology, Organic Chemistry and Catalysis, Julianalaan 136, 2628 BL Delft, The Netherlands
Published Online: 2009-01-01 | DOI: https://doi.org/10.1351/pac200072071233

The key to waste minimization in fine chemicals manufacture is the widespread substitution of classical organic syntheses employing stoichiometric amounts of inorganic reagents with cleaner, catalytic alternatives. The E factors (by waste per kg product) of chemical processes increase dramatically on going downstream from bulk to fine chemicals and pharmaceuticals, mainly owing to the use of "stoichiometric" methods. The concept of atom efficiency is a useful tool for rapid evaluation of the amount of waste generated by alternative processes. The general theme of atom-efficient, catalytic processes is illustrated with industrially relevant examples. These include catalysis by solid acids and bases, catalytic reductions and oxidations, catalytic C_C bond formation, asymmetric catalysis, biocatalysis, and catalysis in novel media (aqueous and fluorous biphasic systems, supercritical fluids, and ionic liquids).

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    2010, 29, 122, S. 5096 [Crossref], CaoJun-Jie, ZhouFeng, ZhouJian, Angewandte Chemie, Angew Chem, 15213757, Improving the Atom Efficiency of the Wittig Reaction by a “Waste as Catalyst/Co-catalyst” Strategy

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    2010, 24, 2010, S. 4719 [Crossref], PatilNitin T., LakshmiPediredla G. V. V., SinghVipender, European Journal of Organic Chemistry, Eur J Org Chem, 10990690, AuI-Catalyzed Direct Hydroamination/Hydroarylation and Double Hydroamination of Terminal Alkynes

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About the article

Published Online: 2009-01-01

Published in Print: 2000-01-01



Citation Information: Pure and Applied Chemistry, ISSN (Online) 1365-3075, ISSN (Print) 0033-4545, DOI: https://doi.org/10.1351/pac200072071233. Export Citation

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