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Pure and Applied Chemistry

The Scientific Journal of IUPAC

Ed. by Burrows, Hugh / Stohner, Jürgen


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1365-3075
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Volume 79, Issue 11

Issues

Catalysis of nanosized Pd metal catalyst deposited on Ti-containing zeolite by a photo-assisted deposition (PAD) method

Hiromi Yamashita
  • Corresponding author
  • Division of Materials and Manufacturing Science, Graduate School of Engineering, Osaka University, 2-1 Yamada-oka, Suita, Osaka 565-0871, Japan
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/ Yuki Miura
  • Corresponding author
  • Division of Materials and Manufacturing Science, Graduate School of Engineering, Osaka University, 2-1 Yamada-oka, Suita, Osaka 565-0871, Japan
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/ Kohsuke Mori
  • Corresponding author
  • Division of Materials and Manufacturing Science, Graduate School of Engineering, Osaka University, 2-1 Yamada-oka, Suita, Osaka 565-0871, Japan
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/ Sayoko Shironita
  • Corresponding author
  • Division of Materials and Manufacturing Science, Graduate School of Engineering, Osaka University, 2-1 Yamada-oka, Suita, Osaka 565-0871, Japan
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/ Yosuke Masui
  • Corresponding author
  • Division of Materials and Manufacturing Science, Graduate School of Engineering, Osaka University, 2-1 Yamada-oka, Suita, Osaka 565-0871, Japan
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/ Naoki Mimura
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  • Division of Materials and Manufacturing Science, Graduate School of Engineering, Osaka University, 2-1 Yamada-oka, Suita, Osaka 565-0871, Japan
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/ Tetsutaro Ohmichi
  • Corresponding author
  • Division of Materials and Manufacturing Science, Graduate School of Engineering, Osaka University, 2-1 Yamada-oka, Suita, Osaka 565-0871, Japan
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/ Takao Sakata
  • Corresponding author
  • Research Center for Ultra-High Voltage Electron Microscopy, Osaka University, 7-1 Mihogaoka, Ibaraki, Osaka 567-0047, Japan
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/ Hirotaro Mori
  • Corresponding author
  • Research Center for Ultra-High Voltage Electron Microscopy, Osaka University, 7-1 Mihogaoka, Ibaraki, Osaka 567-0047, Japan
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Published Online: 2009-01-01 | DOI: https://doi.org/10.1351/pac200779112095

Using a photo-assisted deposition (PAD) method, nanosized Pd metal can be highly dispersed on Ti-containing silicalite zeolite (TS-1) under UV-light irradiation (PAD-Pd/TS-1). The nanosized Pd metal was deposited directly on the photo-excited tetrahedrally coordinated titanium oxide species (tetra-Ti-oxide) of TS-1 zeolite. Under the flow of H2 and O2 in water solvent, the efficient formation of H2O2 could be observed by the PAD-Pd/TS-1 catalyst under mild reaction conditions (ambient temperature and atmospheric pressure). Furthermore, the presence of phenol in this reaction system led to the formation of the products from the partial oxidation of phenol with the formed H2O2.

Keywords: nano Pd metal; photo-assisted deposition; single-site photocatalysts; zeolites

Conference

International IUPAC Conference on Green-Sustainable Chemistry, IUPAC International Conference on Green Chemistry, ICGC, Green Chemistry , 1st, Dresden, Germany, 2006-09-10–2006-09-15

References

About the article

Published Online: 2009-01-01

Published in Print: 2007-01-01


Citation Information: Pure and Applied Chemistry, Volume 79, Issue 11, Pages 2095–2100, ISSN (Online) 1365-3075, ISSN (Print) 0033-4545, DOI: https://doi.org/10.1351/pac200779112095.

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