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Pure and Applied Chemistry

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Volume 79, Issue 8 (Jan 2007)

Issues

Structure, magnetism, and thermodynamics of the novel rare earth-based R5T4 intermetallics

V. K. Pecharsky
  • Corresponding author
  • Ames Laboratory of the U.S. Department of Energy and Department of Materials Science and Engineering, Iowa State University, Ames, IA 50011-3020, USA
/ K. A. Gschneidner
  • Corresponding author
  • Ames Laboratory of the U.S. Department of Energy and Department of Materials Science and Engineering, Iowa State University, Ames, IA 50011-3020, USA
Published Online: 2009-01-01 | DOI: https://doi.org/10.1351/pac200779081383

After approximately 30 years of dormancy, the binary, ternary, and multicomponent intermetallic compounds of rare earth metals (R) with the group 14 elements (T) at the R5T4 stoichiometry have become a goldmine for materials science, condensed matter physics, and solid-state chemistry. In addition to providing numerous opportunities to clarify elusive structure-property relationships, the R5T4 compounds may soon be developed into practical materials by exploiting their unique sensitivity toward a variety of chemical and physical triggers. The distinctiveness of this series is in the remarkable flexibility of the chemical bonding between well-defined, self-assembled, subnanometer-thick slabs and the resultant magnetic, transport, and thermodynamic properties of the R5T4 compounds that can be controlled by varying either or both R and T, including mixed rare earth elements on the R-sites and different group 14 (and 13 or 15) elements occupying the T-sites. In addition to chemical means, the interslab interactions are tunable by temperature, pressure, and magnetic field. Presently, a substantial, yet far from complete, body of knowledge exists about the Gd compounds with T = Si and Ge. In contrast, only a little is known about the physics and chemistry of R5T4 alloys with other lanthanides, while compounds with T = Sn and Pb remain virtually unexplored.

Keywords: crystal structures; experimental thermodynamic properties; intermetallic compounds; magnetic properties; phase relationships; structure–property relationships

Conference

International Conference on Chemical Thermodynamics (ICCT-19), Conference on Chemical Thermodynamics, ICCT, Chemical Thermodynamics, 19th, Boulder, CO, USA, 2006-07-30–2006-08-04

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About the article

Published Online: 2009-01-01

Published in Print: 2007-01-01


Citation Information: Pure and Applied Chemistry, ISSN (Online) 1365-3075, ISSN (Print) 0033-4545, DOI: https://doi.org/10.1351/pac200779081383. Export Citation

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C. L. Wang, J. D. Zou, J. Liu, Y. Mudryk, K. A. Gschneidner, Y. Long, V. Smetana, G. J. Miller, and V. K. Pecharsky
Journal of Applied Physics, 2013, Volume 113, Number 17, Page 17A904
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Y. Mudryk, V. K. Pecharsky, and K. A. Gschneidner
Journal of Applied Physics, 2013, Volume 113, Number 17, Page 17E104
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Jinlei Yao, Yuemei Zhang, Peng L. Wang, Laura Lutz, Gordon J. Miller, and Yurij Mozharivskyj
Physical Review Letters, 2013, Volume 110, Number 7
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Suheyla Yuce, Maria Barrio, Baris Emre, Enric Stern-Taulats, Antoni Planes, Josep-Lluís Tamarit, Yaroslav Mudryk, Karl A. Gschneidner, Vitalij K. Pecharsky, and Lluís Mañosa
Applied Physics Letters, 2012, Volume 101, Number 7, Page 071906
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J. H. Belo, A. M. Pereira, J. P. Araújo, C. de la Cruz, A. M. dos Santos, J. N. Gonçalves, V. S. Amaral, L. Morellon, M. R. Ibarra, P. A. Algarabel, and C. Magen
Physical Review B, 2012, Volume 86, Number 1
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Ya. Mudryk, Niraj K. Singh, V. K. Pecharsky, D. L. Schlagel, T. A. Lograsso, and K. A. Gschneidner
Physical Review B, 2012, Volume 85, Number 9
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J.H. Belo, A.M. Pereira, J. Ventura, G.N.P. Oliveira, J.P. Araújo, P.B. Tavares, L. Fernandes, P.A. Algarabel, C. Magen, L. Morellon, and M.R. Ibarra
Journal of Alloys and Compounds, 2012, Volume 529, Page 89
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S. Vélez, J. M. Hernandez, A. García-Santiago, J. Tejada, V. K. Pecharsky, K. A. Gschneidner, D. L. Schlagel, T. A. Lograsso, and P. V. Santos
Physical Review B, 2012, Volume 85, Number 5
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K.A. Gschneidner and V.K. Pecharsky
International Journal of Refrigeration, 2008, Volume 31, Number 6, Page 945
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Ya. Mudryk, D. Paudyal, V. K. Pecharsky, and K. A. Gschneidner
Physical Review B, 2012, Volume 85, Number 1
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N. Marcano, P. A. Algarabel, J. Rodríguez Fernández, C. Magén, L. Morellón, Niraj K. Singh, D. L. Schlagel, K. A. Gschneidner, V. K. Pecharsky, and M. R. Ibarra
Physical Review B, 2012, Volume 85, Number 2
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Hui Wang, Fei Wang, Karah Jones, and Gordon J. Miller
Inorganic Chemistry, 2011, Volume 50, Number 24, Page 12714
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K.A. Gschneidner, Ya. Mudryk, A.T. Becker, and J.L. Larson
Calphad, 2009, Volume 33, Number 1, Page 8
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Yaroslav Mudryk, Vitalij K. Pecharsky, and Karl A. Gschneidner Jr.
Zeitschrift für anorganische und allgemeine Chemie, 2011, Volume 637, Number 13, Page 1948
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S. M. Disseler, J. N. Svensson, S. C. Peter, C. P. Byers, C. Baines, A. Amato, S. R. Giblin, P. Carretta, and M. J. Graf
Physical Review B, 2011, Volume 84, Number 17
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M. Zou, V.K. Pecharsky, K.A. Gschneidner, D.L. Schlagel, and T.A. Lograsso
Journal of Alloys and Compounds, 2009, Volume 488, Number 2, Page 550
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Durga Paudyal, Y. Mudryk, V. K. Pecharsky, and K. A. Gschneidner
Physical Review B, 2011, Volume 84, Number 1
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J D Moore, G K Perkins, K Morrison, L Ghivelder, M K Chattopadhyay, S B Roy, P Chaddah, K A Gschneidner Jr, V K Pecharsky, and L F Cohen
Journal of Physics: Condensed Matter, 2008, Volume 20, Number 46, Page 465212
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S.B. Roy, P. Chaddah, V.K. Pecharsky, and K.A. Gschneidner
Acta Materialia, 2008, Volume 56, Number 20, Page 5895
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Rabindra Nath Mahato, K. Sethupathi, V. Sankaranarayanan, R. Nirmala, A. K. Nigam, and S. K. Malik
Journal of Applied Physics, 2011, Volume 109, Number 7, Page 07E319
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Durga Paudyal, Ya. Mudryk, V. K. Pecharsky, and K. A. Gschneidner
Physical Review B, 2010, Volume 82, Number 14
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B. R. Hansen, C. R. H. Bahl, L. Theil Kuhn, A. Smith, K. A. Gschneidner, and V. K. Pecharsky
Journal of Applied Physics, 2010, Volume 108, Number 4, Page 043923
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Y. Mudryk, D. Paudyal, V. K. Pecharsky, K. A. Gschneidner, S. Misra, and G. J. Miller
Physical Review Letters, 2010, Volume 105, Number 6
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Durga Paudyal, Y. Mudryk, V. K. Pecharsky, S. Misra, G. J. Miller, and K. A. Gschneidner
Journal of Applied Physics, 2010, Volume 107, Number 9, Page 09A908
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A. S. Chernyshov, Ya. Mudryk, D. Paudyal, V. K. Pecharsky, K. A. Gschneidner, D. L. Schlagel, and T. A. Lograsso
Physical Review B, 2009, Volume 80, Number 18
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Z. W. Ouyang, H. Nojiri, S. Yoshii, G. H. Rao, Y. C. Wang, V. K. Pecharsky, and K. A. Gschneidner
Physical Review B, 2008, Volume 77, Number 18
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Sumohan Misra, Eric T. Poweleit, and Gordon J. Miller
Zeitschrift für anorganische und allgemeine Chemie, 2009, Volume 635, Number 6-7, Page 889
[38]
Durga Paudyal, V K Pecharsky, and K A Gschneidner Jr
Journal of Physics: Condensed Matter, 2008, Volume 20, Number 23, Page 235235
[39]
V. K. Pecharsky and K. A. Jr. Gschneidner
ChemInform, 2007, Volume 38, Number 52

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