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Pure and Applied Chemistry

The Scientific Journal of IUPAC

Ed. by Burrows, Hugh / Stohner, Jürgen


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Volume 81, Issue 9

Issues

Modification of molecular organization of polymers by gas sorption: Thermodynamic aspects and industrial applications

Séverine A. E. Boyer
  • Corresponding author
  • Centre for Material Forming, CEMEF (CNRS UMR 7635), Mines ParisTech, 06904 Sophia Antipolis, France
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/ Takeshi Yamada
  • Corresponding author
  • Institute for Solid State Physics, The University of Tokyo, Tokyo, Kashiwa 277-8581, Japan
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/ Hirohisa Yoshida
  • Corresponding author
  • Graduate School of Environmental Science, Tokyo Metropolitan University, Hachiouji Tokyo 198-0397, Japan
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/ Jean-Pierre E. Grolier
  • Corresponding author
  • Laboratory of Thermodynamics of Solutions and Polymers, Blaise Pascal University, 63177 Aubière, France
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Published Online: 2009-08-19 | DOI: https://doi.org/10.1351/PAC-CON-08-11-09

In polymer science, gas–polymer interactions play a central role for the development of new polymeric structures for specific applications. This is typically the case for polymer foaming and for self-assembling of nanoscale structures where the nature of the gas and the thermodynamic conditions are essential to control. An important applied field where gas sorption in polymers has to be documented through intensive investigations concerns the (non)-controlled solubilization of light gases in the polymers serving, for example, in the oil industry for the transport of petroleum fluids. An experimental set-up coupling a vibrating-wire (VW) detector and a pVT technique has been used to simultaneously evaluate the amount of gas entering a polymer under controlled temperature and pressure and the concomitant swelling of the polymer. Scanning transitiometry has been used to determine the interaction energy during gas sorption in different polymers; the technique was also used to determine the thermophysical properties of polymers submitted to gas sorption. The role of the pressurizing fluid has been documented in terms of the influence of pressure, temperature, and nature of the fluid.

Keywords: gas sorption; high pressure; polymers; scanning transitiometry; vibrating-wire technique

Conference

International Symposium on Solubility Phenomena and Related Equilibrium Processes (ISSP-13), International Symposium on Solubility Phenomena, ISSP, Solubility Phenomena, 13th, Dublin, Ireland, 2008-07-27–2008-07-31

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About the article

Published Online: 2009-08-19

Published in Print: 2009-08-19


Citation Information: Pure and Applied Chemistry, Volume 81, Issue 9, Pages 1603–1614, ISSN (Online) 1365-3075, ISSN (Print) 0033-4545, DOI: https://doi.org/10.1351/PAC-CON-08-11-09.

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