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Pure and Applied Chemistry

The Scientific Journal of IUPAC

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Volume 82, Issue 11

Issues

Total synthesis of biologically active alkaloids using transition metals

Ronny Forke
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  • Department of Chemistry, Technical University of Dresden, Bergstrasse 66, 01069 Dresden, Germany
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/ Konstanze K. Gruner
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  • Department of Chemistry, Technical University of Dresden, Bergstrasse 66, 01069 Dresden, Germany
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/ Kerstin E. Knott
  • Corresponding author
  • Department of Chemistry, Technical University of Dresden, Bergstrasse 66, 01069 Dresden, Germany
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/ Stefan Auschill
  • Corresponding author
  • Department of Chemistry, Technical University of Dresden, Bergstrasse 66, 01069 Dresden, Germany
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/ Sameer Agarwal
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  • Department of Chemistry, Technical University of Dresden, Bergstrasse 66, 01069 Dresden, Germany
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/ René Martin
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  • Department of Chemistry, Technical University of Dresden, Bergstrasse 66, 01069 Dresden, Germany
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/ Markus Böhl
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  • Institute of Zoology, Technical University of Dresden, Zellescher Weg 20b, 01217 Dresden, Germany
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/ Sabine Richter
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  • Institute of Zoology, Technical University of Dresden, Zellescher Weg 20b, 01217 Dresden, Germany
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/ Georgios Tsiavaliaris
  • Corresponding author
  • Institute for Biophysical Chemistry, Hannover Medical School, 30623 Hannover, Germany
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/ Roman Fedorov
  • Corresponding author
  • Institute for Biophysical Chemistry, Hannover Medical School, 30623 Hannover, Germany
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/ Dietmar J. Manstein
  • Corresponding author
  • Institute for Biophysical Chemistry, Hannover Medical School, 30623 Hannover, Germany
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/ Herwig O. Gutzeit
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  • Institute of Zoology, Technical University of Dresden, Zellescher Weg 20b, 01217 Dresden, Germany
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/ Hans-Joachim Knölker
  • Corresponding author
  • Department of Chemistry, Technical University of Dresden, Bergstrasse 66, 01069 Dresden, Germany
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Published Online: 2010-08-06 | DOI: https://doi.org/10.1351/PAC-CON-09-12-15

We have developed efficient synthetic routes to heterocyclic ring systems using transition metals (palladium, iron, and silver). Recent applications of this chemistry to the total synthesis of biologically active alkaloids include carbazole alkaloids (pityriazole, euchrestifoline, the antiostatins), crispine A, pentabromo- and pentachloropseudilin. The two latter alkaloids represent a novel class of myosin ATPase inhibitors that led to the discovery of a new allosteric binding site of the protein.

Keywords: alkaloids; iron; myosin; palladium; silver

Conference

International Symposium on Novel Materials and Their Synthesis (NMS-V) and the 19th International Symposium on Fine Chemistry and Functional Polymers (FCFP-XIX), Novel Materials and their Synthesis, NMS, Novel Materials and their Synthesis, 5th, Shanghai, China, 2009-10-18–2009-10-22

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About the article

Published Online: 2010-08-06

Published in Print: 2010-08-06


Citation Information: Pure and Applied Chemistry, Volume 82, Issue 11, Pages 1975–1991, ISSN (Online) 1365-3075, ISSN (Print) 0033-4545, DOI: https://doi.org/10.1351/PAC-CON-09-12-15.

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