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Pure and Applied Chemistry

The Scientific Journal of IUPAC

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Volume 82, Issue 2 (Nov 2009)

Issues

Terminology for reversible-deactivation radical polymerization previously called "controlled" radical or "living" radical polymerization (IUPAC Recommendations 2010)

Aubrey D. Jenkins / Richard G. Jones / Graeme Moad
  • Corresponding author
  • CSIRO Molecular and Health Technologies, Bag 10, Clayton South, VIC 3169, Australia
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
Published Online: 2009-11-18 | DOI: https://doi.org/10.1351/PAC-REP-08-04-03

This document defines terms related to modern methods of radical polymerization, in which certain additives react reversibly with the radicals, thus enabling the reactions to take on much of the character of living polymerizations, even though some termination inevitably takes place. In recent technical literature, these reactions have often been loosely referred to as, inter alia, "controlled", "controlled/living", or "living" polymerizations. The use of these terms is discouraged. The use of "controlled" is permitted as long as the type of control is defined at its first occurrence, but the full name that is recommended for these polymerizations is "reversible-deactivation radical polymerization".

Keywords: active-dormant equilibria; aminoxyl-mediated; AMRP; atom transfer; ATRP; chain polymerization; controlled; degenerative transfer; DTRP; IUPAC Polymer Division; living; nitroxide-mediated; NMRP; radical; RAFT; reversible-addition-fragmentation chain transfer; reversible-deactivation

Project Year: 2002, Project Code: 2002-006-2-400

References

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    IUPAC. Compendium of Chemical Terminology, 2nd ed. (the “Gold Book”). Compiled by A. D. McNaught and A. Wilkinson. Blackwell Scientific Publications, Oxford (1997). XML on-line corrected version: http://goldbook.iupac.org (2006–) created by M. Nic, J. Jirat, B. Kosata; updates compiled by A. Jenkins.Google Scholar

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    , T. R. Darling, T. P. Davis, M. Fryd, A. A. Gridnev, D. M. Haddleton, S. D. Ittel, R. R. Matheson, G. Moad, E. Rizzardo. J. Polym. Sci., Part A: Polym. Chem. 38, 1706 (2000).CrossrefGoogle Scholar

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    , A. D. Jenkins, P. Kratochvíl, R. F. T. Stepto, U. W. Suter. Pure Appl. Chem. 68, 2287 (1996).CrossrefGoogle Scholar

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    , S. Penczek, G. Moad. Pure Appl. Chem. 80, 2163 (2008).CrossrefGoogle Scholar

About the article

Published Online: 2009-11-18

Published in Print: 2009-11-18


Citation Information: Pure and Applied Chemistry, ISSN (Online) 1365-3075, ISSN (Print) 0033-4545, DOI: https://doi.org/10.1351/PAC-REP-08-04-03.

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