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Pure and Applied Chemistry

The Scientific Journal of IUPAC

Ed. by Burrows, Hugh / Stohner, Jürgen

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Volume 83, Issue 4

Issues

Tuning plasmon transitions and their applications in organic photochemistry

Juan C. Scaiano
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ José C. Netto-Ferreira
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Emilio Alarcon
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Paul Billone
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Carlos J. Bueno Alejo
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Charles-Oneil L. Crites
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Matthew Decan
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Chiara Fasciani
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ María González-Béjar
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Geniece Hallett-Tapley
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Michel Grenier
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Katherine L. McGilvray
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Natalia L. Pacioni
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Andrea Pardoe
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Laetitia René-Boisneuf
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Rachel Schwartz-Narbonne
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ M. Jazmín Silvero
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Kevin G. Stamplecoskie
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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/ Tse-Luen Wee
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  • Department of Chemistry, Centre for Catalysis Research and Innovation, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada
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Published Online: 2011-03-14 | DOI: https://doi.org/10.1351/PAC-CON-11-01-09

The ketone-photoinduced formation of Au, Ag, and Cu nanoparticles from their corresponding ions in solution has been carried out using benzoin photoinitiators. Ketones are good photosensitizers for nanoparticle synthesis not because of the energy they can absorb or deliver, but rather because of the reducing free radicals they can generate. Efficient photochemical nanoparticle generation thus requires a careful selection of substrates and experimental conditions such that free radical generation occurs with high quantum efficiency, where metal ion precursors do not inhibit radical formation. A key consideration to achieve nanoparticle synthesis with short exposure times is to minimize excited-state quenching by metal ions. Applications of nanostructures in catalysis require control of the nanoparticle characteristics, such as dimension, morphology, and surface properties. Part of this article describes the strategies to modify photochemically prepared particles. Finally, we illustrate some of the nanoparticle applications that interest us, with some emphasis on plasmon-mediated processes.

Keywords: catalysis; nanoparticles; noble metals; photochemistry; photoinitiator; plasmon

Conference

IUPAC Symposium on Photochemistry, International Symposium on Photochemistry, PHOTO, Photochemistry, XXIIIrd, Ferrara, Italy, 2010-07-11–2010-07-16

References

About the article

Published Online: 2011-03-14

Published in Print: 2011-03-14


Citation Information: Pure and Applied Chemistry, Volume 83, Issue 4, Pages 913–930, ISSN (Online) 1365-3075, ISSN (Print) 0033-4545, DOI: https://doi.org/10.1351/PAC-CON-11-01-09.

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