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Radiochimica Acta

International Journal for chemical aspects of nuclear science and technology

Editor-in-Chief: Qaim, Syed M.

12 Issues per year


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Source Normalized Impact per Paper (SNIP) 2017: 0.869

Online
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2193-3405
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Volume 89, Issue 8

Issues

The migration of radionuclides 237Np, 238Pu and 241Am in a weak loess aquifer: A field column experiment

L. Chunli / W. Zhiming / Li Shushen / Y. Yuee / J. Hong / Li Bing / J. Ling / W. Ling / L. Dan / Du Zhongde / G. Zhiming
Published Online: 2009-09-25 | DOI: https://doi.org/10.1524/ract.2001.89.8.519

The migration of radionuclides 237Np, 238Pu and 241Am in a weak loess aquifer were investigated in-situ with a bisectional experimental column. The experimental column was constructed by connecting 2 undisturbed aquifer medium columns together and inserted into the aquifer horizontally through holes pre-prepared in the wall of a vertical experimental shaft in an Underground Research Facility at the CIRP´s field test site. Quartz containing radionuclides 3H, 237Np, 238Pu and 241Am was introduced as a point source at the center of the experimental column. Outflow water of the experimental column was collected and 3H in the outflow was determined for calculating the water flow velocity through the experimental column. The experimental column was cut into slices of 0.3 cm long and the radioactivity of 237Np, 238Pu and 241Am in the sliced soil samples was analyzed when the experiment was completed.

The water flow velocity in the experimental column was calculated as 1.15±0.05 cm/d. The activity distribution of 237Np, 238Pu and 241Am in the experimental column indicate that each radionuclide has a very strong activity distribution region adjacent to the source introduction point and decreases abruptly as the distance increases. In addition there are other secondary activity distribution regions with different strength and widths. The calculated apparent distribution coefficients of the main specie of these radionuclides is (8.90±1.51)×102 ml/g for 237Np, (9.48±1.61)×102 ml/g for 238Pu and (9.79±1.66)×102 ml/g for 241Am.

About the article

Published Online: 2009-09-25

Published in Print: 2001-08-01


Citation Information: Radiochimica Acta, Volume 89, Issue 8, Pages 519–522, ISSN (Online) 2193-3405, ISSN (Print) 0033-8230, DOI: https://doi.org/10.1524/ract.2001.89.8.519.

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