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Radiochimica Acta

International Journal for chemical aspects of nuclear science and technology

Editor-in-Chief: Qaim, Syed M.

12 Issues per year


IMPACT FACTOR 2016: 1.271
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CiteScore 2017: 1.22

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Source Normalized Impact per Paper (SNIP) 2017: 0.869

Online
ISSN
2193-3405
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Volume 90, Issue 7

Issues

Photofission of 209Bi at intermediate energies

H. Haba / M. Kasaoka / M. Igarashi / K. Washiyama / H. Matsumura / Y. Oura / S. Shibata / K. Sakamoto / M. Furukawa / I. Fujiwara
Published Online: 2009-09-25 | DOI: https://doi.org/10.1524/ract.2002.90.7_2002.371

Summary

The reaction yields of 63 radionuclides with the mass number A = 56 − 135 produced in the photofission of 209Bi by bremsstrahlung of end-point energies (E0) from 450 to 1100 MeV have been measured using a catcher foil technique with the aid of intensive chemical separation. The charge distribution was well reproduced by a Gaussian function with the most probable charge (Zp) expressed by a linear function of A, i.e., Zp = RA + S, and with the A-independent full width at half maximum (FWHMCD). The charge distribution parameters R, S and FWHMCD were independent of E0 above 600 MeV, reflecting the resonance nature in photonuclear reactions at intermediate energies. The weighted mean values at E0 ≥ 600 MeV were R = 0.421 ± 0.001, S = 0.6 ± 0.1 and FWHMCD = 2.1 ± 0.1 charge unit (c.u.). The numbers of pre- and post-fission neutrons were deduced to be νpre = 12 ± 1 and νpost = 1.4 ± 0.3, respectively, assuming the Unchanged Charge Distribution (UCD). Based on the charge distribution parameters, the symmetric mass yield distributions with the most probable mass Ap of 96 ± 1 mass unit (m.u.) and the width FWHMMD of 33 ± 1 m.u. were also obtained. The characteristics of the charge and mass yield distributions are discussed by referring to those for 197Au based on the results of calculations using the Photon-induced Intranuclear Cascade Analysis code combined with the Generalized Evaporation Model (PICA3/GEM).

About the article

Received: 2001-10-17

Accepted: 2002-03-25

Published Online: 2009-09-25

Published in Print: 2002-07-01


Citation Information: Radiochimica Acta, Volume 90, Issue 7, Pages 371–382, ISSN (Online) 2193-3405, ISSN (Print) 0033-8230, DOI: https://doi.org/10.1524/ract.2002.90.7_2002.371.

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[1]
H. Haba, K. Sakamoto, M. Igarashi, M. Kasaoka, K. Washiyama, H. Matsumura, Y. Oura, S. Shibata, M. Furukawa, and I. Fujiwara
Czechoslovak Journal of Physics, 2003, Volume 53, Number S1, Page A265

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