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Zeitschrift für Physikalische Chemie

International journal of research in physical chemistry and chemical physics

Editor-in-Chief: Rademann, Klaus


IMPACT FACTOR 2018: 0.975
5-year IMPACT FACTOR: 1.021

CiteScore 2018: 1.20

SCImago Journal Rank (SJR) 2018: 0.327
Source Normalized Impact per Paper (SNIP) 2018: 0.391

Online
ISSN
2196-7156
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Volume 229, Issue 10-12

Issues

On the Relation between Population Kinetics and State-to-State Rate Coefficients for Vibrational Energy Transfer

Elena I. Dashevskaya
  • Schulich Faculty of Chemistry, Technion – Israel Institute of Technology, 32000, Haifa, Israel
  • Max-Planck-Institut für Biophysikalische Chemie, Am Fassberg 11, D-37077 Göttingen, Germany
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Ilya Litvin
  • Institut für Physikalische Chemie, Universität Göttingen, Tammannstrasse 6, D-37077 Göttingen, Germany
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Evgeny E. Nikitin
  • Corresponding author
  • Schulich Faculty of Chemistry, Technion – Israel Institute of Technology, 32000, Haifa, Israel
  • Max-Planck-Institut für Biophysikalische Chemie, Am Fassberg 11, D-37077 Göttingen, Germany
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  • Other articles by this author:
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Published Online: 2015-08-28 | DOI: https://doi.org/10.1515/zpch-2015-0597

Abstract

The relation between time-dependent population of vibrational state and collision-induced state-to-state rate coefficients is discussed within the Landau–Teller kinetic equations for the relaxation of harmonic oscillators in a heat bath. In particular, the increase of the populations in the first and the second vibrational state of an initially cold oscillator shows a considerable variety of its relation to a single Landau–Teller state-to-state rate coefficient. It is suggested that this variety should be kept in mind when experimental studies of the relaxation of specific level are analyzed.

Keywords: Reaction Kinetics

About the article

Accepted: 2015-07-28

Received: 2015-03-20

Published Online: 2015-08-28

Published in Print: 2015-10-28


Citation Information: Zeitschrift für Physikalische Chemie, Volume 229, Issue 10-12, Pages 1561–1574, ISSN (Online) 2196-7156, ISSN (Print) 0942-9352, DOI: https://doi.org/10.1515/zpch-2015-0597.

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[1]
E. I. Dashevskaya, I. Litvin, E. E. Nikitin, and J. Troe
The Journal of Chemical Physics, 2018, Volume 149, Number 1, Page 014301

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