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Zeitschrift für Physikalische Chemie

International journal of research in physical chemistry and chemical physics

Editor-in-Chief: Rademann, Klaus


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Volume 232, Issue 7-8

Issues

Chemically Modified Silica Materials as Model Systems for the Characterization of Water-Surface Interactions

Martin Brodrecht
  • Eduard-Zintl-Institute of Inorganic and Physical Chemistry, Technical University of Darmstadt, Alarich-Weiss-Str. 8, D-64287 Darmstadt, Germany
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Bharti Kumari
  • Eduard-Zintl-Institute of Inorganic and Physical Chemistry, Technical University of Darmstadt, Alarich-Weiss-Str. 8, D-64287 Darmstadt, Germany
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Hergen Breitzke
  • Eduard-Zintl-Institute of Inorganic and Physical Chemistry, Technical University of Darmstadt, Alarich-Weiss-Str. 8, D-64287 Darmstadt, Germany
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Torsten Gutmann
  • Eduard-Zintl-Institute of Inorganic and Physical Chemistry, Technical University of Darmstadt, Alarich-Weiss-Str. 8, D-64287 Darmstadt, Germany
  • Other articles by this author:
  • De Gruyter OnlineGoogle Scholar
/ Gerd Buntkowsky
  • Corresponding author
  • Eduard-Zintl-Institute of Inorganic and Physical Chemistry, Technical University of Darmstadt, Alarich-Weiss-Str. 8, D-64287 Darmstadt, Germany
  • Email
  • Other articles by this author:
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Published Online: 2018-01-10 | DOI: https://doi.org/10.1515/zpch-2017-1059

Abstract

A series of novel functionalized mesoporous silica-based materials with well-defined pore diameters, surface functionalization and surface morphology is synthesized by co-condensation or grafting techniques and characterized by solid-state NMR spectroscopy, DNP enhanced solid state-NMR and thermodynamic techniques. These materials are employed as host-systems for small-guest molecules like water, small alcohols, carbonic acids, small aromatic molecules, binary mixtures and others. The phase-behavior of these confined guests is studied by combinations of one dimensional solid-state NMR techniques (1H MAS, 2H-line shape analysis, 13C CPMAS) and two-dimensional correlation experiments like 1H-29Si- solid-state HETCOR.

Keywords: confinement; micro-phase separation; solid-state-NMR

References

  • 1.

    M. S. Morey, A. Davidson, G. D. Stucky, J. Porous Mat. 5 (1998) 195.CrossrefGoogle Scholar

  • 2.

    H. T. Chen, S. Huh, J. W. Wiench, M. Pruski, V. S. Y. Lin, J. Am. Chem. Soc. 127 (2005) 13305.CrossrefPubMedGoogle Scholar

  • 3.

    X. G. Wang, K. S. K. Lin, J. C. C. Chan, S. F. Cheng, J. Phys. Chem. B 109 (2005) 1763.CrossrefPubMedGoogle Scholar

  • 4.

    A. Vinu, K. Z. Hossain, K. Ariga, J. Nanosci. Nanotec. 5 (2005) 347.CrossrefGoogle Scholar

  • 5.

    A. Vinu, M. Miyahara, K. Ariga, J. Nanosci. Nanotec. 6 (2006) 1510.CrossrefGoogle Scholar

  • 6.

    J. S. Beck, J. C. Vartuli, W. J. Roth, M. E. Leonowicz, C. T. Kresge, K. D. Schmitt, C. T. W. Chu, D. H. Olson, E. W. Sheppard, S. B. Mccullen, J. B. Higgins, J. L. Schlenker, J. Am. Chem. Soc. 114 (1992) 10834.CrossrefGoogle Scholar

  • 7.

    A. Sayari, S. Hamoudi, Chem. Mater. 13 (2001) 3151.CrossrefGoogle Scholar

  • 8.

    M. Vallet-Regi, A. Ramila, R. Del Real, J. Pérez-Pariente, Chem. Mater. 13 (2001) 308.CrossrefGoogle Scholar

  • 9.

    P. Selvam, S. K. Bhatia, C. G. Sonwane, Ind. Eng. Chem. Res. 40 (2001) 3237.CrossrefGoogle Scholar

  • 10.

    A. Schreiber, I. Ketelsen, G. H. Findenegg, Phys. Chem. Chem. Phys. 3 (2001) 1185.CrossrefGoogle Scholar

  • 11.

    F. Schüth, W. Schmidt, Adv. Eng. Mat. 4 (2002) 269.CrossrefGoogle Scholar

  • 12.

    S. R. Hall, D. Walsh, D. Green, R. Oreffo, S. Mann, J. Mater. Chem. 13 (2003) 186.CrossrefGoogle Scholar

  • 13.

    T. Linssen, K. Cassiers, P. Cool, E. Vansant, Adv. Colloid Interface Sci. 103 (2003) 121.CrossrefPubMedGoogle Scholar

  • 14.

    A. Adamczyk, Y. Xu, B. Walaszek, F. Roelofs, T. Pery, K. Pelzer, K. Philippot, B. Chaudret, H.-H. Limbach, H. Breitzke, Top. Catal. 48 (2008) 75.CrossrefGoogle Scholar

  • 15.

    R. Mellaerts, J. A. G. Jammaer, M. Van Speybroeck, H. Chen, J. Van Humbeeck, P. Augustijns, G. Van den Mooter, J. A. Martens, Langmuir 24 (2008) 8651.CrossrefPubMedGoogle Scholar

  • 16.

    T. Ukmar, T. Cendak, M. Mazaj, V. Kaucic, G. Mali, J. Phys. Chem. C 116 (2012) 2662.Google Scholar

  • 17.

    A. Grünberg, H. Breitzke, G. Buntkowsky, Solid State NMR of Immobilized Catalysts and Nanocatalysts, In Spectroscopic Properties of Inorganic and Organometallic Compounds: Techniques, Materials and Applications, J. Yarwood, R. Douthwaite, S. Duckett, Eds. Royal Society of Chemistry, Cambridge, UK (2012), P. 289.Google Scholar

  • 18.

    T. Gutmann, A. Grünberg, N. Rothermel, M. Werner, M. Srour, S. Abdulhussain, S. Tan, Y. Xu, H. Breitzke, G. Buntkowsky, Solid State Nucl. Mag. 55–56 (2013) 1.Google Scholar

  • 19.

    D. Y. Zhao, J. L. Feng, Q. S. Huo, N. Melosh, G. H. Fredrickson, B. F. Chmelka, G. D. Stucky, Science 279 (1998) 548.CrossrefPubMedGoogle Scholar

  • 20.

    D. Y. Zhao, Q. S. Huo, J. L. Feng, B. F. Chmelka, G. D. Stucky, J. Am. Chem. Soc. 120 (1998) 60246.Google Scholar

  • 21.

    L. D. Gelb, K. E. Gubbins, R. Radhakrishnan, M. Sliwinska-Bartkowiak, Rep. Prog. Phys. 62 (1999) 1573.CrossrefGoogle Scholar

  • 22.

    U. Ciesla, F. Schüth, Microporous Mesoporous Mater. 27 (1999) 131.CrossrefGoogle Scholar

  • 23.

    M. Werner, N. Rothermel, H. Breitzke, T. Gutmann, G. Buntkowsky, Isr. J. Chem. 54 (2014) 60.CrossrefGoogle Scholar

  • 24.

    Y. P. Xu, T. Watermann, H. H. Limbach, T. Gutmann, D. Sebastiani, G. Buntkowsky, Phys. Chem. Chem. Phys. 16 (2014) 9327.CrossrefPubMedGoogle Scholar

  • 25.

    A. S. Maria Chong, X. S. Zhao, J. Phys. Chem. B 107 (2003) 12650.CrossrefGoogle Scholar

  • 26.

    T. Yokoi, H. Yoshitake, T. Tatsumi, J. Mater. Chem. 14 (2004) 951.CrossrefGoogle Scholar

  • 27.

    M. Kahse, M. Werner, S. Zhao, M. Hartmann, G. Buntkowsky, R. Winter, J. Phys. Chem. C 118 (2014) 21523.CrossrefGoogle Scholar

  • 28.

    C. Alba-Simionesco, B. Coasne, G. Dosseh, G. Dudziak, K. Gubbins, R. Radhakrishnan, M. Sliwinska-Bartkowiak, J. Phys. Condens. Mat. 18 (2006) 15.Google Scholar

  • 29.

    E. Gedat, A. Schreiber, J. Albrecht, I. Shenderovich, G. Findenegg, H.-H. Limbach, G. Buntkowsky, J. Phys. Chem. B 106 (2002) 1977.CrossrefGoogle Scholar

  • 30.

    P. Medick, T. Blochowicz, M. Vogel, E. Roessler, J. Non-Cryst. Solids 307 (2002) 565.Google Scholar

  • 31.

    G. Dosseh, Y. Xia, C. Alba-Simionesco, J. Phys. Chem. 107 (2003) 6445.CrossrefGoogle Scholar

  • 32.

    S. A. Lusceac, C. Koplin, P. Medick, M. Vogel, N. Brodie-Linder, C. LeQuellec, C. Alba-Simionesco, E. A. Roessler, J. Phys. Chem. B 108 (2004) 16601.CrossrefGoogle Scholar

  • 33.

    G. Höhne, W. F. Hemminger, H.-J. Flammersheim, Differential Scanning Calorimetry, Springer, Berlin Heidelberg (2003).Google Scholar

  • 34.

    W. F. Hemminger, H. K. Cammenga, Methoden der thermischen Analyse, Springer Berlin (1989).Google Scholar

  • 35.

    M. Schoen, S. H. L. Klapp, Nanoconfined Fluids. Soft Matter Between Two and Three Dimensions Volume 24, John Wiley & Sons, New York (2007).Google Scholar

  • 36.

    I. Shenderovich, G. Buntkowsky, A. Schreiber, E. Gedat, S. Sharif, J. Albrecht, N. S. Golubev, G. H. Findenegg, H. H. Limbach, J. Phys. Chem. B 107 (2003) 11924.CrossrefGoogle Scholar

  • 37.

    B. Grünberg, T. Emmler, E. Gedat, I. Shenderovich, G. H. Findenegg, H. H. Limbach, G. Buntkowsky, Chem.-Eur. J. 10 (2004) 5689.CrossrefGoogle Scholar

  • 38.

    W. Masierak, T. Emmler, E. Gedat, A. Schreiber, G. H. Findenegg, G. Buntkowsky, J. Phys. Chem. B 108 (2004) 18890.CrossrefGoogle Scholar

  • 39.

    A. Vyalikh, T. Emmler, E. Gedat, I. Shenderovich, G. H. Findenegg, H.-H. Limbach, G. Buntkowsky, Solid State NMR 28 (2005) 117.CrossrefGoogle Scholar

  • 40.

    G. Buntkowsky, H. Breitzke, A. Adamczyk, F. Roelofs, T. Emmler, E. Gedat, B. Grünberg, Y. Xu, H. H. Limbach, I. Shenderovich, A. Vyalikh, G. H. Findenegg, Phys. Chem. Chem. Phys. 9 (2007) 4843.PubMedCrossrefGoogle Scholar

  • 41.

    A. Vyalikh, T. Emmler, B. Grünberg, Y. Xu, I. Shenderovich, G. H. Findenegg, H.-H. Limbach, G. Buntkowsky, Z. für Phys. Chem. 221 (2007) 155.CrossrefGoogle Scholar

  • 42.

    A. Vyalikh, T. Emmler, I. Shenderovich, Y. Zeng, G. H. Findenegg, G. Buntkowsky, Phys. Chem. Chem. Phys. 9 (2007) 2249.CrossrefPubMedGoogle Scholar

  • 43.

    N. de-Sousa-Amadeu, B. Grünberg, J. Frydel, M. Werner, H.-H. Limbach, H. Breitzke, G. Buntkowsky, Z. Phys. Chem. 226 (2012) 1169.CrossrefGoogle Scholar

  • 44.

    S. Jayanthi, M. Werner, Y. Xu, G. Buntkowsky, S. Vega, J. Phys. Chem. C 117 (2013) 13114.CrossrefGoogle Scholar

  • 45.

    M. Sattig, S. Reutter, F. Fujara, M. Werner, G. Buntkowsky, M. Vogel, Phys. Chem. Chem. Phys. 16 (2014) 19229.PubMedCrossrefGoogle Scholar

  • 46.

    M. Werner, A. Heil, N. Rothermel, H. Breitzke, P. B. Groszewicz, A. S. Thankamony, T. Gutmann, G. Buntkowsky, Solid State Nucl. Mag. 72 (2015) 73.CrossrefGoogle Scholar

  • 47.

    A. Barnes, G. De Paepe, P. Van der Wel, K.-N. Hu, C.-G. Joo, V. Bajaj, M. Mak-Jurkauskas, J. Sirigiri, J. Herzfeld, R. Temkin, R. G. Griffin, App. Magn. Res. 34 (2008) 237.CrossrefGoogle Scholar

  • 48.

    A. Lesage, M. Lelli, D. Gajan, M. A. Caporini, V. Vitzthum, P. Mieville, J. Alauzun, A. Roussey, C. Thieuleux, A. Mehdi, G. Bodenhausen, C. Coperet, L. Emsley, J. Am. Chem. Soc. 132 (2010) 15459.PubMedCrossrefGoogle Scholar

  • 49.

    M. Lelli, D. Gajan, A. Lesage, M. A. Caporini, V. Vitzthum, P. Mieville, F. Heroguel, F. Rascon, A. Roussey, C. Thieuleux, M. Boualleg, L. Veyre, G. Bodenhausen, C. Coperet, L. Emsley, J. Am. Chem. Soc. 133 (2011) 2104.CrossrefPubMedGoogle Scholar

  • 50.

    D. Gajan, M. Schwarzwälder, M. P. Conley, W. R. Grüning, A. J. Rossini, A. Zagdoun, M. Lelli, M. Yulikov, G. Jeschke, C. Sauvée, O. Ouari, P. Tordo, L. Veyre, A. Lesage, C. Thieuleux, L. Emsley, C. Copéret, J. Am. Chem. Soc. 135 (2013) 15459.PubMedCrossrefGoogle Scholar

  • 51.

    A. S. L. Thankamony, O. Lafon, X. Lu, F. Aussenac, M. Rosay, J. Trebosc, H. Vezin, J.-P. Amoureux, App. Magn. Res. 43 (2012) 237.CrossrefGoogle Scholar

  • 52.

    M. F. Harrach, B. Drossel, J. Chem. Phys. 140 (2014) 174501.PubMedCrossrefGoogle Scholar

  • 53.

    E. Ackermann, E. M. Weiel, T. Pfaff, B. Drossel, Eur. Phys. J. E 35 (2012) 1.CrossrefGoogle Scholar

  • 54.

    P. v. R. Schleyer, C. Maerker, A. Dransfeld, H. Jiao, N. J. v. E. Hommes, J. Am. Chem. Soc. 118 (1996) 6317.PubMedCrossrefGoogle Scholar

  • 55.

    D. Sebastiani, ChemPhysChem 7 (2006) 164.PubMedCrossrefGoogle Scholar

  • 56.

    D. Sebastiani, K. N. Kudin, ACS Nano 2 (2008) 661.PubMedCrossrefGoogle Scholar

  • 57.

    M. Weigler, M. Brodrecht, H. Breitzke, F. Dietrich, M. Sattig, G. Buntkowsky, M. Vogel, Z. Phys. Chem. 232 (2018) 1041.Google Scholar

  • 58.

    S. Mann, Biomineralization: Principles and Concepts in Bioinorganic Materials Chemistry Volume 5, Oxford University Press on Demand, Oxford (2001).Google Scholar

  • 59.

    M. J. Duer, J. Magn. Reson. 253 (2015) 98.CrossrefPubMedGoogle Scholar

  • 60.

    M. Sumper, E. Brunner, Chembiochem 9 (2008) 1187.CrossrefPubMedGoogle Scholar

  • 61.

    N. Poulsen, M. Sumper, N. Kröger, Proc. Natl. Acad. Sci. USA 100 (2003) 12075.CrossrefGoogle Scholar

  • 62.

    E. Brunner, C. Groger, K. Lutz, P. Richthammer, K. Spinde, M. Sumper, Appl. Microbiol. Biotechnol. 84 (2009) 607.CrossrefPubMedGoogle Scholar

  • 63.

    N. Almqvist, Y. Delamo, B. L. Smith, N. H. Thomson, A. Bartholdson, R. Lal, M. Brzezinski, P. K. Hansma, J. Microsc. 202 (2001) 518.PubMedCrossrefGoogle Scholar

  • 64.

    N. Nassif, J. Livage, Chem. Soc. Rev. 40 (2011) 849.PubMedCrossrefGoogle Scholar

  • 65.

    Z. Zhou, F. Piepenbreier, V. R. R. Marthala, K. Karbacher, M. Hartmann, Catal. Today 243 (2014) 173.Google Scholar

  • 66.

    M. Hartmann, X. Kostrov, Chem. Soc. Rev. 42 (2013) 6277.CrossrefPubMedGoogle Scholar

  • 67.

    I. Matlahov, Y. Geiger, G. Goobes, Phys. Chem. Chem. Phys. 16 (2014) 9031.CrossrefPubMedGoogle Scholar

  • 68.

    S. Jayanthi, B. Chatterjee, S. Raghothama, Biopolymers 91 (2009) 851.CrossrefPubMedGoogle Scholar

  • 69.

    A. Zagdoun, G. Casano, O. Ouari, G. Lapadula, A. J. Rossini, M. Lelli, M. Baffert, D. Gajan, L. Veyre, W. E. Maas, M. Rosay, R. T. Weber, C. Thieuleux, C. Coperet, A. Lesage, P. Tordo, L. Emsley, J. Am. Chem. Soc. 134 (2012) 2284.CrossrefPubMedGoogle Scholar

  • 70.

    B. Kumari, D. John, P. Hoffmann, A. Spende, M. E. Toimil-Molares, C. Trautmann, C. Hess, P. Ruff, R. Stark, M. Schulze, G. Buntkowsky, A. Andrieu-Brunsen, T. Gutmann, Z. für Phys. Chem. (2018) this issue.Google Scholar

  • 71.

    M. Brodrecht, E. Klotz, C. Lederle, H. Breitzke, B. Stühn, M. Vogel, G. Buntkowsky, Z. für Phys. Chem. (2018) this issue.Google Scholar

  • 72.

    J. A. Lee, H. Rösner, J. F. Corrigan, Y. Huang, J. Phys. Chem. C 115 (2011) 4738.Google Scholar

  • 73.

    B. Grünberg, A. Grünberg, H.-H. Limbach, G. Buntkowsky, App. Magn. Res. 44 (2013) 189.CrossrefGoogle Scholar

  • 74.

    E. Roessler, M.Taupitz, K. Börner, M. Schulz, H. M. Vieth, J. Chem. Phys. 92 (1990) 5847.CrossrefGoogle Scholar

  • 75.

    M. Ebener, G. Vonfircks, H. Günther, Helv. Chim. Acta 74 (1991) 1296.CrossrefGoogle Scholar

  • 76.

    M. Ebener, V. Francke, H. Günther, Fresenius J. Anal Chem. 357 (1997) 505.CrossrefGoogle Scholar

  • 77.

    G. von Fircks, H. Hausmann, V. Francke, H. Günther, J. Org. Chem. 62 (1997) 5074.CrossrefGoogle Scholar

  • 78.

    H. Günther, S. Oepen, M. Ebener, V. Francke, Magn. Reson. Chem. 37 (1999) 142.CrossrefGoogle Scholar

  • 79.

    M. F. Harrach, B. Drossel, W. Winschel, T. Gutmann, G. Buntkowsky, J. Phys. Chem. C 119 (2015) 28961.CrossrefGoogle Scholar

  • 80.

    B. J. van Rossum, H. Förster, H. J. M. de Groot, J. Magn. Reson. 124 (1997) 516.CrossrefGoogle Scholar

About the article

Received: 2017-10-20

Accepted: 2017-12-07

Published Online: 2018-01-10

Published in Print: 2018-07-26


Citation Information: Zeitschrift für Physikalische Chemie, Volume 232, Issue 7-8, Pages 1127–1146, ISSN (Online) 2196-7156, ISSN (Print) 0942-9352, DOI: https://doi.org/10.1515/zpch-2017-1059.

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