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Zeitschrift für Physikalische Chemie

International journal of research in physical chemistry and chemical physics

Editor-in-Chief: Rademann, Klaus

12 Issues per year


IMPACT FACTOR 2017: 1.144
5-year IMPACT FACTOR: 1.144

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2196-7156
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Volume 232, Issue 9-11

Issues

Single Particle Spectroscopy of Radiative Processes in Colloid-to-Film-Coupled Nanoantennas

Max J. Schnepf
  • Leibniz Institute of Polymer Research (IPF), Institute of Physical Chemistry and Polymer Physics, Hohe Str. 6, 01069 Dresden, Germany
  • Other articles by this author:
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/ Yannic Brasse
  • Leibniz Institute of Polymer Research (IPF), Institute of Physical Chemistry and Polymer Physics, Hohe Str. 6, 01069 Dresden, Germany
  • Cluster of Excellence Center for Advancing Electronics Dresden (CFAED), Technische Universität Dresden, Dresden, Germany
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/ Fabian R. Goßler
  • Leibniz Institute of Polymer Research (IPF), Institute of Physical Chemistry and Polymer Physics, Hohe Str. 6, 01069 Dresden, Germany
  • Cluster of Excellence Center for Advancing Electronics Dresden (CFAED), Technische Universität Dresden, Dresden, Germany
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/ Anja Maria Steiner
  • Leibniz Institute of Polymer Research (IPF), Institute of Physical Chemistry and Polymer Physics, Hohe Str. 6, 01069 Dresden, Germany
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/ Julian Obermeier
  • Lehrstuhl Experimentalphysik III, Department of Physics, University Bayreuth, Universitätsstraße 30, 95447 Bayreuth, Germany
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/ Markus Lippitz
  • Lehrstuhl Experimentalphysik III, Department of Physics, University Bayreuth, Universitätsstraße 30, 95447 Bayreuth, Germany
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/ Andreas Fery
  • Corresponding author
  • Leibniz Institute of Polymer Research (IPF), Institute of Physical Chemistry and Polymer Physics, Hohe Str. 6, 01069 Dresden, Germany
  • Cluster of Excellence Center for Advancing Electronics Dresden (CFAED), Technische Universität Dresden, Dresden, Germany
  • Physical Chemistry of Polymeric Materials, Technische Universität Dresden, Dresden, Germany
  • Email
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/ Tobias A.F. König
  • Corresponding author
  • Leibniz Institute of Polymer Research (IPF), Institute of Physical Chemistry and Polymer Physics, Hohe Str. 6, 01069 Dresden, Germany
  • Cluster of Excellence Center for Advancing Electronics Dresden (CFAED), Technische Universität Dresden, Dresden, Germany
  • Email
  • Other articles by this author:
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Published Online: 2018-04-14 | DOI: https://doi.org/10.1515/zpch-2018-1109

Abstract

We present a fluorescent emitter (rhodamine B) coupled to a dielectric or metallic interface as well as a metallic cavity to study their radiative decay processes. Supported by finite-difference time-domain (FDTD) simulations, we correlate the non-radiative and radiative decay rates with the absorption and scattering cross section efficiencies, respectively. On a single particle level, we use atomic force microscopy (AFM), scanning electron microscopy (SEM), scattering spectroscopy, fluorescence life time imaging (FLIM) and time-correlated single photon counting (TCSPC) to evaluate the enhanced fluorescence decay at the same location. With this study, we show a colloidal gain material, which can be integrated into lattices using existing directed self-assembled methods to study their coherent energy transfer.

This article offers supplementary material which is provided at the end of the article.

Keywords: enhancement; fluorescence; life time; metallic film; nanoparticle; quantum emitter; spectroscopy

Contribution to: Geburtstagsband Eychmüller

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About the article

aMax J. Schnepf and Yannic Brasse: These authors contributed equally.


Received: 2018-01-15

Accepted: 2018-03-20

Published Online: 2018-04-14

Published in Print: 2018-08-28


Citation Information: Zeitschrift für Physikalische Chemie, Volume 232, Issue 9-11, Pages 1593–1606, ISSN (Online) 2196-7156, ISSN (Print) 0942-9352, DOI: https://doi.org/10.1515/zpch-2018-1109.

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[2]
Nadja C. Bigall and Nikolai Gaponik
Zeitschrift für Physikalische Chemie, 2018, Volume 232, Number 9-11, Page 1263

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